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I made my own rip of this game (PAL version) with no freezing problems. As I recall, I downsampled all music to 22050 stereo, and downsampled a few videos. I believe the cause of the freezing problem would be this, it just can't stream video and audio fast enough, no matter the sort order (I used the original sort order). Using a 99 minute wouldn't help, CD-R is just plain slow compared to GD-ROM.
Not sure about your mkisofs problem, what are sorting with? What's your command line?
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