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That must be DVD-Roms you have there. You have to rip these first and do some work on them before you can burn them. For every game there is a special tutorial means way to do so.
Check out the following sites I hope they can give you information, tutorials and tools:
www.ps2ownz.com
www.gamecopyworld.com (use the search function)
www.ps2.sgt-dan.com
www.megagames.com
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